Publications

2013

• Cell death induced on cell cultures and nude mouse skin by non-thermal, nanosecond-pulsed generated plasma
  
  • Duval Arnaud
  • Marinov Ilya
  • Bousquet Guilhem
  • Gapihan Guillaume
  • Starikovskaia Svetlana
  • Rousseau Antoine
  • Janin Anne
  PLoS ONE, Public Library of Science, 2013, 8 (12), pp.e83001. Non-thermal plasmas are gaseous mixtures of molecules, radicals, and excited species with a small proportion of ions and energetic electrons. Non-thermal plasmas can be generated with any high electro-magnetic field. We studied here the pathological effects, and in particular cell death, induced by nanosecond-pulsed high voltage generated plasmas homogeneously applied on cell cultures and nude mouse skin. In vitro, Jurkat cells and HMEC exhibited apoptosis and necrosis, in dose-dependent manner. In vivo, on nude mouse skin, cell death occurred for doses above 113 J/cm(2) for the epidermis, 281 J/cm(2) for the dermis, and 394 J/cm(2) for the hypodermis. Using electron microscopy, we characterized apoptosis for low doses and necrosis for high doses. We demonstrated that these effects were not related to thermal, photonic or pH variations, and were due to the production of free radicals. The ability of cold plasmas to generate apoptosis on cells in suspension and, without any sensitizer, on precise skin areas, opens new fields of application in dermatology for extracorporeal blood cell treatment and the eradication of superficial skin lesions. (10.1371/journal.pone.0083001)
  DOI : 10.1371/journal.pone.0083001
• Fine-structure-resolved electron collisions from chlorine atoms in the (3p<SUP>5</SUP>)<SUP>2</SUP>P<SUB>3/2</SUB><SUP>o</SUP> and (3p<SUP>5</SUP>)<SUP>2</SUP>P<SUB>1/2</SUB><SUP>o</SUP> states
  
  • Wang Yang
  • Zatsarinny Oleg
  • Bartschat Klaus
  • Booth Jean-Paul
  Physical Review A : Atomic, molecular, and optical physics [1990-2015], American Physical Society, 2013, 87, pp.022703. The B-spline R-matrix method is employed to calculate elastic electron scattering from chlorine atoms in the (3p5)2P3/2,1/2o states and electron-induced collisions between these two finestructure levels. The polarizability of the target states is accounted for by including polarized pseudostates in the close-coupling expansion, while relativistic effects are treated at the level of the semirelativistic Breit-Pauli approximation. We find the Ramsauer minimum in the elastic channels at a significantly lower projectile energy (&#8776;0.2 eV) than previous calculations, due to an apparent strong sensitivity of the theoretical predictions on the details of the model, especially the target structure. The present results are relevant to the determination of chlorine atomic densities in Cl2-containing industrial plasma etch reactors. (10.1103/PhysRevA.87.022703)
  DOI : 10.1103/PhysRevA.87.022703
• Vibrational relaxation of N2 on catalytic surfaces studied by infrared titration with time resolved Quantum Cascade Laser diagnostics
  
  • Marinov Daniil
  • Guaitella Olivier
  • Lopatik D.
  • Hübner M.
  • Ionikh Y.
  • Roepcke J.
  • Rousseau Antoine
  , 2013.
• Electrical characteristics of micro-hollow cathode discharges
  
  • Lazzaroni Claudia
  • Chabert Pascal
  Journal of Physics D: Applied Physics, IOP Publishing, 2013, 46, pp.455203. A cathode sheath model of micro-hollow cathode discharges is proposed to calculate the voltagecurrent characteristics and discuss the physics of the discharge resistance. Three different approaches are compared: (i) a self-consistent model where the electric field is determined self-consistently with the electron flux, (ii) a matrix sheath model where the electric field profile in the sheath is imposed, (iii) a constant electric field model where the electric field in the sheath is assumed to be equal to a constant fraction of the electric field at the cathode. The sheath size is found to decrease with the pressure, the voltage and the secondary emission coefficient. There is a strong effect of the secondary emission coefficient and the pressure on the voltagecurrent characteristics. The discharge resistance is found to be several hundreds of k&#937; and decreases with the discharge current, the pressure and the secondary emission coefficient. A comparison between the matrix sheath model and experiments suggests that both the secondary emission coefficient and the surface area on which the current is collected at the cathode increase with the discharge current. This increase is related to a transition between a discharge confined in the hole at low current and a plasma abruptly expanded on the cathode backside at higher current. (10.1088/0022-3727/46/45/455203)
  DOI : 10.1088/0022-3727/46/45/455203
• A comparison of bow shock models with Cluster observations during low Alfvén Mach number magnetic clouds
  
  • Turc Lucile
  • Fontaine Dominique
  • Savoini Philippe
  • Hietala H.
  • Kilpua E. K. J.
  Annales Geophysicae, European Geosciences Union, 2013, 31 (6), pp.1011-019. Magnetic clouds (MCs) are very geoeffective solar wind structures. Their properties in the interplanetary medium have been extensively studied, yet little is known about their characteristics in the Earth's magnetosheath. The Cluster spacecraft offer the opportunity to observe MCs in the magnetosheath, but before MCs reach the magnetosphere, their structure is altered when they interact with the terrestrial bow shock (BS). The physics taking place at the BS strongly depends on ΘBn, the angle between the shock normal and the interplanetary magnetic field. However, in situ observations of the BS during an MC's crossing are seldom available. In order to relate magnetosheath observations to solar wind conditions, we need to rely on a model to determine the shock's position and normal direction. Yet during MCs, the models tend to be less accurate, because the Alfvén Mach number (MA) is often significantly lower than in regular solar wind. On the contrary, the models are generally optimised for high MA conditions. In this study, we compare the predictions of four widely used models available in the literature (Wu et al., 2000; Chapman and Cairns, 2003; Jeřáb et al., 2005; Měrka et al., 2005b) to Cluster's dayside BS crossings observed during five MC events. Our analysis shows that the ΘBn angle is well predicted by all four models. On the other hand, the Jeřáb et al. (2005) model yields the best estimates of the BS position during low MA MCs. The other models locate the BS either too far from or too close to Earth. The results of this paper can be directly used to estimate the BS parameters in all studies of MC interaction with Earth's magnetosphere. (10.5194/angeo-31-1011-2013)
  DOI : 10.5194/angeo-31-1011-2013
• A study of helium atmospheric-pressure guided streamers for potential biological applications
  
  • Gazeli Kristacq
  • Noel Cédric
  • Clement Franck
  • Dauge C.
  • Svarnas P.
  • Belmonte Thierry
  Plasma Sources Science and Technology, IOP Publishing, 2013, 22 (2), pp.025020. The origin of differences in the rotational temperatures of various molecules and ions (N-2(+)(B), OH(A) and N-2(C)) is studied in helium atmospheric-pressure guided streamers. The rotational temperature of N-2(+)(B) is room temperature. It is estimated from the emission band of the first negative system at 391.4 nm, and it is governed by the temperature of N-2(X) in the surrounding air. N-2(X) is ionized by direct electron impact in the outer part of the plasma. N-2(+)(B) is deactivated by collisions with N-2 and O-2. The rotational temperature of OH(A), estimated from the OH band at 306.4 nm, is slightly higher than that of N-2(+)(B). OH(A) is excited by electron impact with H2O during the first 100 ns of the applied voltage pulse. Next, OH(A) is produced by electron impact with OH(X) created by the quenching of OH(A) by N-2 and O-2. H2O diffuses deeper than N-2 into the plasma ring and the rotational temperature of OH(A) is slightly higher than that of N-2(+)(B). The rotational temperature of N-2(C), estimated from the emission of the second positive system at 315.9 nm, is governed by its collisions with helium. The gas temperature of helium at the beginning of the pulse is predicted to be several hundred kelvin higher than room temperature. (10.1088/0963-0252/22/2/025020)
  DOI : 10.1088/0963-0252/22/2/025020
• In Situ Cassini Spacecraft Observations of Turbulence in Saturn's Magnetosheath
  
  • Hadid L. Z.
  • Sahraoui Fouad
  • Retinò Alessandro
  • Modolo Ronan
  • Canu Patrick
  • Jackman C. M.
  • Masters A.
  • Dougherty M. K.
  • Gurnett D. A.
  , 2013, 8, pp.EPSC2013-1056. Throughout this work we investigate, the properties of turbulence in the Magnetosheath of Saturn. To do so, we computed Power Spectral Densities (PSD) based on Cassini interplanetary magnetic field data between 2004 and 2007. As a preliminary result, we show the absence of the Kolmogorov scale ~ f-5/3 in the inertial range whereas only the f-1 scale is present.
• Atmospheric Pressure Townsend Discharges in nitrogen with small admixtures of oxygen: discussion on the origin of the memory effect
  
  • Naudé Nicolas
  • Bouzidi Mohamed Cherif
  • Dang V.S.
  • Dang van Sung Mussard Marguerite
  • Puechagut Loïc
  • Belinger Antoine
  • Ségur Pierre
  • Gherardi Nicolas
  , 2013.
• Generation mechanism of the whistler-mode waves in the plasma sheet prior to magnetic reconnection
  
  • Wei X.H.
  • Cao J.B.
  • Zhou G.C.
  • Fu H.S.
  • Santolík O.
  • Rème H.
  • Dandouras I.
  • Cornilleau-Wehrlin Nicole
  • Fazakerley A.
  Advances in Space Research, Elsevier, 2013, 52 (1), pp.205-210. The whistler-mode waves and electron temperature anisotropy play a key role prior to and during magnetic reconnection. On August 21, 2002, the Cluster spacecrafts encountered a quasi-collisionless magnetic reconnection event when they crossed the plasma sheet. Prior to the southward turning of magnetospheric magnetic field and high speed ion flow, the whistler-mode waves and positive electron temperature anisotropy are simultaneously observed. Theoretic analysis shows that the electrons with positive temperature anisotropy can excite the whistler-mode waves via cyclotron resonances. Using the data of particles and magnetic field, we estimated the whistler-mode wave growth rate and the ratio of whistler-mode growth rate to wave frequency. They are 0.0016fce (Electron cyclotron frequency) and 0.0086fce, respectively. Therefore the whistler-mode waves can grow quickly in the current sheet. The combined observations of energetic electron beams and waves show that after the southward turning of magnetic field, energetic electrons in the reconnection process are accelerated by the whistler-mode waves. (10.1016/j.asr.2013.02.016)
  DOI : 10.1016/j.asr.2013.02.016
• Reinterpretation of Slowdown of Solar Wind Mean Velocity in Nonlinear Structures Observed Upstream of Earth's Bow Shock
  
  • Parks G. K.
  • Lee E.
  • Lin N.
  • Fu S. Y.
  • Mccarthy M.
  • Cao J.B.
  • Hong J.
  • Liu Y.
  • Shi J. K.
  • Goldstein M. L.
  • Canu Patrick
  • Dandouras I.
  • Rème H.
  The Astrophysical Journal Letters, Bristol : IOP Publishing, 2013, 771, pp.L39. Two of the many features associated with nonlinear upstream structures are (1) the solar wind (SW) mean flow slows down and deviates substantially and (2) the temperature of the plasma increases in the structure. In this Letter, we show that the SW beam can be present throughout the entire upstream event maintaining a nearly constant beam velocity and temperature. The decrease of the velocity is due to the appearance of new particles moving in the opposite direction that act against the SW beam and reduce the mean velocity as computed via moments. The new population, which occupies a larger velocity space, also contributes to the second moment, increasing the temperature. The new particles include the reflected SW beam at the bow shock and another population of lower energies, accelerated nearby at the shock or at the boundary of the nonlinear structures. (10.1088/2041-8205/771/2/L39)
  DOI : 10.1088/2041-8205/771/2/L39
• SPACE RESEARCH IN AFRICA SOME ACHIEVEMENTS FROM 2007 to 2012
  
  • Amory-Mazaudier Christine
  • Fleury Rolland
  Sun and Geosphere, BBC SWS Regional Network, 2013, 1, pp.ISSN : I819-0839. This article presents the results of a research network Europe Africa established in 1995 after the International Electrojet Equatorial Year (1992-1994). During the last decade, this research network has been involved in two international projects: the International Heliophysical Year (2007-2009) and International Space Weather Initiative (2010-2012).The participation in these international projects increased the number of PhD and multiplied the number of scientific papers. Many scientific results have been obtained. Teaching and working methods have been also developed. We emphasize in this article the last two points.
• In situ observations of high-Mach number collisionless shocks in space plasmas
  
  • Masters A.
  • Stawarz L.
  • Fujimoto M.
  • Schwartz S. J.
  • Sergis N.
  • Thomsen M. F.
  • Retinò Alessandro
  • Hasegawa H.
  • Zieger B.
  • Lewis G. R.
  • Coates A. J.
  • Canu Patrick
  • Dougherty M. K.
  Plasma Physics and Controlled Fusion, IOP Publishing, 2013, 55 (12), pp.124035. Shock waves are widespread in collisionless space plasmas throughout the Universe. How particles are accelerated at these shocks has been the subject of much research attention. The dominant source of the high-energy particles that pervade our Galaxy (cosmic rays) is thought to be the high-Mach number collisionless shocks that form around young supernova remnants, but it is unclear how much the lower Mach number collisionless shock waves frequently encountered by spacecraft in Solar System space plasmas can tell us about particle acceleration in the higher Mach number regime. Here we review recent studies of the shock wave that stands in the solar wind in front of the planet Saturn (Saturn's bow shock), based on Cassini spacecraft observations. This review represents a new direction of shock physics research, with the potential to bridge the gap between Solar System and astrophysical shocks. These studies have confirmed that Saturn's bow shock is one of the strongest shocks in the Solar System, and a recent discovery indicates that electron acceleration at high-Mach numbers may occur irrespective of the upstream magnetic field geometry. This is important because astrophysical shocks can often only be studied remotely via emissions associated with accelerated electrons. We discuss possible future directions of this emerging sub-field of collisionless space plasma shock physics. (10.1088/0741-3335/55/12/124035)
  DOI : 10.1088/0741-3335/55/12/124035
• Interplanetary Nanodust Detection by the Solar Terrestrial Relations Observatory/WAVES Low Frequency Receiver
  
  • Le Chat G.
  • Zaslavsky A.
  • Meyer-Vernet N.
  • Issautier K.
  • Belheouane S.
  • Pantellini F.
  • Maksimovic M.
  • Zouganelis I.
  • Bale S. D.
  • Kasper J. C.
  Solar Physics, Springer Verlag, 2013, 286 (2), pp.549-559. New measurements using radio and plasma-wave instruments in interplanetary space have shown that nanometer-scale dust, or nanodust, is a significant contributor to the total mass in interplanetary space. Better measurements of nanodust will allow us to determine where it comes from and the extent to which it interacts with the solar wind. When one of these nanodust grains impacts a spacecraft, it creates an expanding plasma cloud, which perturbs the photoelectron currents. This leads to a voltage pulse between the spacecraft body and the antenna. Nanodust has a high charge/mass ratio, and therefore can be accelerated by the interplanetary magnetic field to the speed of the solar wind: significantly faster than the Keplerian orbital speeds of heavier dust. The amplitude of the signal induced by a dust grain grows much more strongly with speed than with mass of the dust particle. As a result, nanodust can produce a strong signal despite its low mass. The WAVES instruments on the twin Solar TErrestrial RElations Observatory spacecraft have observed interplanetary nanodust particles since shortly after their launch in 2006. After describing a new and improved analysis of the last five years of STEREO/WAVES Low Frequency Receiver data, we present a statistical survey of the nanodust characteristics, namely the rise time of the pulse voltage and the flux of nanodust. We show that previous measurements and interplanetary dust models agree with this survey. The temporal variations of the nanodust flux are also discussed. (10.1007/s11207-013-0268-x)
  DOI : 10.1007/s11207-013-0268-x
• A double-plasma source of continuous bipolar ion-ion beam
  
  • Dudin S.V.
  • Rafalskyi D.V.
  Applied Physics Letters, American Institute of Physics, 2013, 102, pp.034102. A double-plasma source capable of the generation of a continuous bipolar ion-ion beam is described. The quasi-neutral ion-ion flow to an extraction electrode is formed in the system containing primary inductively coupled plasma separated from a secondary plasma by an electrostatic grid-type filter. The total current of each ion species to the 250&#8201;mm diameter extraction electrode is about 80&#8201;mA; the electron current does not exceed 30% of the ion current. Method of positive/negative ion current ratio control is proposed, allowing the ion currents ratio variation in wide range. (10.1063/1.4788711)
  DOI : 10.1063/1.4788711
• Radiation from Ag High Energy Density Z-pinch Plasmas with Applications to Lasing
  
  • Weller M. E.
  • Safronova Alla S.
  • Kantsyrev Viktor L.
  • Esaulov A. A.
  • Shrestha Ishor
  • Apruzese J. P.
  • Giuliani J. L.
  • Chuvatin Alexandre S.
  • Stafford A.
  • Keim S. F.
  • Shlyaptseva V. V.
  • Osborne Glenn C.
  • Petkov E. E.
  , 2013.
• Azimuthal directions of equatorial noise propagation determined using 10 years of data from the Cluster spacecraft
  
  • Nemec F.
  • Santolík O.
  • Pickett J. S.
  • Hrbackova Z.
  • Cornilleau-Wehrlin Nicole
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118, pp.7160-7169. Equatorial noise (EN) emissions are electromagnetic waves at frequencies between the proton cyclotron frequency and the lower hybrid frequency routinely observed within a few degrees of the geomagnetic equator at radial distances from about 2 to 6 R<SUB>E</SUB>. They propagate in the extraordinary (fast magnetosonic) mode nearly perpendicularly to the ambient magnetic field. We conduct a systematic analysis of azimuthal directions of wave propagation, using all available Cluster data from 2001 to 2010. Altogether, combined measurements of the Wide-Band Data and Spectrum Analyzer of the Spatio-Temporal Analysis of Field Fluctuations instruments allowed us to determine azimuthal angle of wave propagation for more than 100 EN events. It is found that the observed propagation pattern is mostly related to the plasmapause location. While principally isotropic azimuthal directions of EN propagation were detected inside the plasmasphere, wave propagation in the plasma trough was predominantly found directed to the West or East, perpendicular to the radial direction. The observed propagation pattern can be explained using a simple propagation analysis, assuming that the emissions are generated close to the plasmapause. (10.1002/2013JA019373)
  DOI : 10.1002/2013JA019373
• Multi-dipolar microwave plasmas and their application to negative ion production
  
  • Béchu Stéphane
  • Soum-Glaude A.
  • Bès A.
  • Lacoste A.
  • Svarnas P.
  • Aleiferis S.
  • Ivanov Jr. A.A.
  • Bacal M.
  Physics of Plasmas, American Institute of Physics, 2013, 20, pp.101601. (10.1063/1.4823466)
  DOI : 10.1063/1.4823466
• ROLE OF REACTOR CAPACITANCE ON THE PROPAGATION OF IONISATION WAVES
  
  • Guaitella Olivier
  • Sobota Ana
  • Rousseau Antoine
  , 2013.
• Direction for the future - Successive acceleration of positive and negative ions applied to space propulsion
  
  • Aanesland Ane
  • Bredin Jérôme
  • Popelier Lara
  • Chabert Pascal
  , 2013 (CERN-2013-007).
• Nonturbulent stabilization of ion fluxes by the fan instability
  
  • Krafft C.
  • Volokitin A.
  Physics Letters A, Elsevier, 2013, 377 (16-17), pp.1189-1198. Resonant interactions between energetic ion fluxes and wave packets they excite through fan instability are studied using self-consistent 3D simulations to explain the nonlinear wave-particle mechanisms at work and to estimate the energy lost by the flux and its sharing between wave emission and particle heating. The saturation of waves and the relaxation of particles are studied over long time periods. The ions are not only diffusing in the waves but are also trapped simultaneously by several potential wells of large amplitude overlapping waves. Estimates of the ion heating energy and rate are given and compared with space observations. (10.1016/j.physleta.2013.03.011)
  DOI : 10.1016/j.physleta.2013.03.011
• Dipolarization fronts as a consequence of transient reconnection: In situ evidence
  
  • Fu H.S.
  • Cao J.B.
  • Khotyaintsev Y. V.
  • Sitnov M. I.
  • Runov A.
  • Fu S. Y.
  • Hamrin M.
  • André M.
  • Retinò Alessandro
  • Ma Y. D.
  • Lu H. Y.
  • Wei X.H.
  • Huang S. Y.
  Geophysical Research Letters, American Geophysical Union, 2013, 40 (23), pp.6023-6027. Dipolarization fronts (DFs) are frequently detected in the Earth's magnetotail from XGSM&#8201;=&#8201;&#8722;30 RE to XGSM&#8201;=&#8201;&#8722;7 RE. How these DFs are formed is still poorly understood. Three possible mechanisms have been suggested in previous simulations: (1) jet braking, (2) transient reconnection, and (3) spontaneous formation. Among these three mechanisms, the first has been verified by using spacecraft observation, while the second and third have not. In this study, we show Cluster observation of DFs inside reconnection diffusion region. This observation provides in situ evidence of the second mechanism: Transient reconnection can produce DFs. We suggest that the DFs detected in the near-Earth region (XGSM&#8201;>&#8201;&#8722;10 RE) are primarily attributed to jet braking, while the DFs detected in the mid- or far-tail region (XGSM&#8201;<&#8201;&#8722;15 RE) are primarily attributed to transient reconnection or spontaneous formation. In the jet-braking mechanism, the high-speed flow pushes the preexisting plasmas to produce the DF so that there is causality between high-speed flow and DF. In the transient-reconnection mechanism, there is no causality between high-speed flow and DF, because the frozen-in condition is violated. (10.1002/2013GL058620)
  DOI : 10.1002/2013GL058620
• Comparison between hybrid and fully kinetic models of asymmetric magnetic reconnection: Coplanar and guide field configurations
  
  • Aunai Nicolas
  • Hesse Michael
  • Zenitani Seiji
  • Kuznetsova M. M.
  • Black Carrie
  • Evans Rebekah
  • Smets Roch
  Physics of Plasmas, American Institute of Physics, 2013, 20, pp.022902. Magnetic reconnection occurring in collisionless environments is a multi-scale process involving both ion and electron kinetic processes. Because of their small mass, the electron scales are difficult to resolve in numerical and satellite data, it is therefore critical to know whether the overall evolution of the reconnection process is influenced by the kinetic nature of the electrons, or is unchanged when assuming a simpler, fluid, electron model. This paper investigates this issue in the general context of an asymmetric current sheet, where both the magnetic field amplitude and the density vary through the discontinuity. A comparison is made between fully kinetic and hybrid kinetic simulations of magnetic reconnection in coplanar and guide field systems. The models share the initial condition but differ in their electron modeling. It is found that the overall evolution of the system, including the reconnection rate, is very similar between both models. The best agreement is found in the guide field system, which confines particle better than the coplanar one, where the locality of the moments is violated by the electron bounce motion. It is also shown that, contrary to the common understanding, reconnection is much faster in the guide field system than in the coplanar one. Both models show this tendency, indicating that the phenomenon is driven by ion kinetic effects and not electron ones. (10.1063/1.4792250)
  DOI : 10.1063/1.4792250
• Asymmetric distribution of reconnection jet fronts in the Jovian nightside magnetosphere
  
  • Kasahara S.
  • Kronberg E. A.
  • Kimura T.
  • Tao C.
  • Badman S. V.
  • Masters A.
  • Retinò Alessandro
  • Krupp N.
  • Fujimoto M.
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118, pp.375-384. Magnetic reconnection plays important roles in mass transport and energy conversion in planetary magnetospheres. It is considered that transient reconnection causes localized auroral arcs or spots in the Jovian magnetosphere, by analogy to the case in the Earth's magnetosphere. However, the local structures of transient reconnection events (i.e., magnetospheric plasma parameters) and their spatial distribution have not been extensively investigated for the Jovian magnetosphere. Here we examine plasma velocity and density during strong north-south magnetic field events in the Jovian nightside magnetosphere, which may be associated with tail reconnection. We find prominent reconnection jet fronts predominantly on the dawnside of the nightside magnetosphere, which would be a signature unique to rotation-dominant planetary magnetospheres. The observed plasma structures are consistent with significant field-aligned currents which would generate localized aurora. (10.1029/2012JA018130)
  DOI : 10.1029/2012JA018130
• Ozone kinetics in low-pressure discharges: vibrationally excited ozone and molecule formation on surfaces
  
  • Marinov Daniil
  • Guerra V.
  • Guaitella Olivier
  • Booth Jean-Paul
  • Rousseau Antoine
  Plasma Sources Science and Technology, IOP Publishing, 2013, 22, pp.055018. A combined experimental and modeling investigation of the ozone kinetics in the afterglow of pulsed direct current discharges in oxygen is carried out. The discharge is generated in a cylindrical silica tube of radius 1 cm, with short pulse durations between 0.5 and 2 ms, pressures in the range 15 Torr and discharge currents &#8764;40120 mA. Time-resolved absolute concentrations of ground-state atoms and ozone molecules were measured simultaneously in situ, by two-photon absorption laser-induced fluorescence and ultraviolet absorption, respectively. The experiments were complemented by a self-consistent model developed to interpret the results and, in particular, to evaluate the roles of vibrationally excited ozone and of ozone formation on surfaces. It is found that vibrationally excited ozone, O&#8727; 3, plays an important role in the ozone kinetics, leading to a decrease in the ozone concentration and an increase in its formation time. In turn, the kinetics of O&#8727; 3 is strongly coupled with those of atomic oxygen and O2(a 1g) metastables. Ozone formation at the wall does not contribute significantly to the total ozone production under the present conditions. Upper limits for the effective heterogeneous recombination probability of O atoms into ozone are established. (10.1088/0963-0252/22/5/055018)
  DOI : 10.1088/0963-0252/22/5/055018
• Secondary electron induced asymmetry in capacitively coupled plasmas
  
  • Lafleur Trevor
  • Chabert Pascal
  • Booth Jean-Paul
  Journal of Physics D: Applied Physics, IOP Publishing, 2013, 46, pp.135201. Using a simple analytical model, together with a 1D particle-in-cell simulation, we show that it is possible to generate an asymmetric plasma response in a sinusoidally excited, geometrically symmetric, capacitively coupled plasma (CCP). The asymmetric response is produced using rf electrodes of differing materials, and hence different secondary electron emission coefficients. This asymmetry in the emission coefficients can produce a significant, measurable dc bias voltage (Vbias /Vrf &#8764; 00.2), together with an asymmetry in the plasma density profiles and ion flux to each electrode. The dc bias formation can be understood from a particle-flux balance applied to each electrode, and results from two main effects: (1) the larger effective ion flux at each electrode due to the emission of secondary electrons and (2) ion-flux multiplication within the sheath due to ionization from these emitted secondary electrons. By making use of an empirical fit to the simulation data, the possibility of non-invasively estimating secondary electron emission coefficients in CCP systems is discussed. (10.1088/0022-3727/46/13/135201)
  DOI : 10.1088/0022-3727/46/13/135201