Publications

2013

• Antisunward structure of thin current sheets in the Earth's magnetotail : Implications of quasi-adiabatic theory
  
  • Malova H. V.
  • Popov V. Y.
  • Delcourt Dominique C.
  • Petrukovich A. A.
  • Zelenyi L. M.
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118. We developed a self-consistent kinetic model of thin current sheets (TCS), taking into account the inhomogeneity of TCS parameters in the antisunward direction. We show that the charged particle dynamics depending on the magnetic field distribution in the downtail direction completely determines the magnetotail equilibrium structure. We demonstrate that transient ions as well as electrons are the main current carriers in this system, but the first ones support mostly the background (1-D) structure of the current sheet. The influence of electrons and quasi-trapped ions is found to vary depending upon downtail distance along the sheet. Assuming the conservation of the so-called quasi-adiabatic invariant, we show that quasi-trapped particles are distributed along the current sheet in such a way that they concentrate in the region with large values of normal magnetic field component. As a result quasi-trapped ions can dominate near the earthward edge of TCS. In contrast, the electron current becomes stronger in the TCS tailward region where the normal magnetic field component becomes weaker, and field line curvature drifts are enhanced. Our quasi-adiabatic model predicts that thin current sheets in the Earth's magnetotail should have weakly 2-D configuration which, similar to its 1-D analog considered earlier, conserves the multiscale matreshka structure with multiple embedded layers. (10.1002/jgra.50390)
  DOI : 10.1002/jgra.50390
• Inner radiation belt particle acceleration and energy structuring by drift resonance with ULF waves during geomagnetic storms
  
  • Delcourt Dominique C.
  • Benoist C.
  • Penou E.
  • Chen Y.
  • Russell C. T.
  • Sauvaud J.-A.
  • Walt M.
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118 (4), pp.1723-1736. Geomagnetic storms are frequently associated with the formation of multiple bands of energetic electrons inside the inner radiation belt at L = 1.1-1.9 and with prominent energy structures of protons inside the slot region at L = 2.2-3.5. These structures typically from 100 keV up to the MeV range result from coherent interactions of energetic particles with quasi-monochromatic ultra-low frequency (ULF) waves. These waves are induced by magnetospheric changes due to the arrival of dense solar material and related nightside injections of particles from the outer magnetosphere that destabilize field lines in the inner magnetosphere down to L = 1.1. Using low-altitude data from the polar orbiting Demeter spacecraft, we perform case and statistical studies of these structures. We show that with such a spacecraft, these structures are best seen near the South Atlantic Anomaly because of lowering of the belt particle mirror point. As evidenced from ground measurements, energy bands are associated with quasi-sinusoidal ULF Pc5 and Pc4 waves with periods in the 1000 s range for L = 1.1-1.9 and in the 60 s range for L = 2.2-3.5. Numerical simulations of the coherent drift resonance of energetic particles with ultra-low frequency waves show how the particles are accelerated and how the observed structures build up. (10.1002/jgra.50125)
  DOI : 10.1002/jgra.50125
• Electron nongyrotropy in the context of collisionless magnetic reconnection
  
  • Aunai Nicolas
  • Hesse Michael
  • Kuznetsova M. M.
  Physics of Plasmas, American Institute of Physics, 2013, 20, pp.2903. Collisionless magnetized plasmas have the tendency to isotropize their velocity distribution function around the local magnetic field direction, i.e., to be gyrotropic, unless some spatial and/or temporal fluctuations develop at the particle gyroscales. Electron gyroscale inhomogeneities are well known to develop during the magnetic reconnection process. Nongyrotropic electron velocity distribution functions have been observed to play a key role in the dissipative process breaking the field line connectivity. In this paper, we present a new method to quantify the deviation of a particle population from gyrotropy. The method accounts for the full 3D shape of the distribution and its analytical formulation allows fast numerical computation. Regions associated with a significant degree of nongyrotropy are shown, as well as the kinetic origin of the nongyrotropy and the fluid signature it is associated with. Using the result of 2.5D Particle-In-Cell simulations of magnetic reconnection in symmetric and asymmetric configurations, it is found that neither the reconnection site nor the topological boundaries are generally associated with a maximized degree of nongyrotropy. Nongyrotropic regions do not correspond to a specific fluid behavior as equivalent nongyrotropy is found to extend over the electron dissipation region as well as in non-dissipative diamagnetic drift layers. The localization of highly nongyrotropic regions in numerical models and their correlation with other observable quantities can, however, improve the characterization of spatial structures explored by spacecraft missions. (10.1063/1.4820953)
  DOI : 10.1063/1.4820953
• Chlorine atom densities in the (3p<SUP>5</SUP>)<SUP>2</SUP> P<SUP>0</SUP><SUB>1/2</SUB> excited spin-orbit state measured by two-photon absorption laser-induced fluorescence in a chlorine inductively coupled plasma
  
  • Sirse Nishant
  • Booth Jean-Paul
  • Chabert Pascal
  • Surzhykov A.
  • Indelicato P.
  Journal of Physics D: Applied Physics, IOP Publishing, 2013, 46 (29), pp.295203. Chlorine atom densities in the spinorbit excited state were measured by two-photon absorption laser-induced fluorescence (TALIF) in an inductively coupled plasma discharge in pure Cl2. The atoms were excited by two photons at 235.702 nm to the state and detected by fluorescence to the (4s) 4P5/2 state at 726 nm. The population of this state relative to that in the ground state, was determined from the relative TALIF signal intensity from the two states, combined with new calculations of the two-photon absorption cross-sections. was found to increase continuously with radio-frequency power (50500 W), whereas with Cl2 pressure (590 mTorr) it passes through a maximum at 10 mTorr, reaching ~30% at 500 W. This maximum corresponds to the maximum of electron density in the discharge. Combining this density ratio measurement with previous measurements of the absolute ground state chlorine atom density [1] allows the absolute spin-orbit excited state density to be estimated. A significant fraction of the total chlorine atom density is in this excited state which should be included in plasma chemistry models. (10.1088/0022-3727/46/29/295203)
  DOI : 10.1088/0022-3727/46/29/295203
• Microsecond ramp compression of a metallic liner driven by a 5 MA current on the SPHINX machine using a dynamic load current multiplier pulse shaping
  
  • d'Almeida Thierry
  • Lassalle Francis
  • Morell Alain
  • Grunenwald Julien
  • Zucchini Frédéric
  • Loyen Arnaud
  • Maysonnave Thomas
  • Chuvatin Alexandre S.
  Physics of Plasmas, American Institute of Physics, 2013, 20 (09), pp.092512. SPHINX is a 6 MA, 1-&#956;s Linear Transformer Driver (LTD) operated by the CEA Gramat (France) and primarily used for imploding Z-pinch loads for radiation effects studies. Among the options that are currently being evaluated to improve the generator performances are an upgrade to a 20&#8201;MA, 1-&#956;s LTD machine and various power amplification schemes, including a compact Dynamic Load Current Multiplier (DLCM). A method for performing magnetic ramp compression experiments, without modifying the generator operation scheme, was developed using the DLCM to shape the initial current pulse in order to obtain the desired load current profile. In this paper, we discuss the overall configuration that was selected for these experiments, including the choice of a coaxial cylindrical geometry for the load and its return current electrode. We present both 3-D Magneto-hydrodynamic and 1D Lagrangian hydrodynamic simulations which helped guide the design of the experimental configuration. Initial results obtained over a set of experiments on an aluminium cylindrical liner, ramp-compressed to a peak pressure of 23&#8201;GPa, are presented and analyzed. Details of the electrical and laser Doppler interferometer setups used to monitor and diagnose the ramp compression experiments are provided. In particular, the configuration used to field both homodyne and heterodyne velocimetry diagnostics in the reduced access available within the liner's interior is described. Current profiles measured at various critical locations across the system, particularly the load current, enabled a comprehensive tracking of the current circulation and demonstrate adequate pulse shaping by the DLCM. The liner inner free surface velocity measurements obtained from the heterodyne velocimeter agree with the hydrocode results obtained using the measured load current as the input. An extensive hydrodynamic analysis is carried out to examine information such as pressure and particle velocity history profiles or magnetic diffusion across the liner. The potential of the technique in terms of applications and achievable ramp pressure levels lies in the prospects for improving the DLCM efficiency through the use of a closing switch (currently under development), reducing the load dimensions and optimizing the diagnostics. (10.1063/1.4823720)
  DOI : 10.1063/1.4823720
• Radial correlation of density fluctuations by coupling IPP and LPP W-band Doppler reflectometers on ASDEX Upgrade
  
  • Hennequin Pascale
  • Happel T.
  • Conway G. D.
  • Honoré Cyrille
  • Vermare Laure
  • Pisarev V.
  • Giacalone J-C.
  • Gürcan Özgür D.
  • Asdex Upgrade Team
  , 2013 (oral).
• Role of the terrestrial bow shock on magnetic clouds structure: 2. 3D analytical MHD model
  
  • Turc Lucile
  • Fontaine Dominique
  • Kilpua E. K. J.
  • Savoini Philippe
  , 2013. Magnetic clouds (MC) figure among the most important drivers of magnetic storms. In the solar wind, they present a very distinctive structure. However, before reaching the magnetosphere, MCs encounter the bow shock which modifies their structure, and therefore may influence their geoeffectivity. In order to understand how the magnetic structure of MCs is altered by the shock, a simple 3D MHD model is used to calculate the magnetic field strength and direction inside the magnetosheath. We present several outputs of the model, corresponding to different MC axis orientations and to different impact parameters. The variation of the magnetic field direction from the solar wind to the magnetosheath appears to be strongly driven by the shock obliquity. Asymmetries due to different shock configurations may arise inside the magnetosheath. Moreover, the Bz component can even reverse in some parts of the magnetosheath. The model outputs are compared with spacecraft observations. Finally, we discuss the impact of our conclusions on MCs geoeffectivity.
• Effects of the surface conductivity and the IMF strength on the dynamics of planetary ions in Mercury's magnetosphere
  
  • Seki Kanako
  • Terada Naoki
  • Yagi Manabu
  • Delcourt Dominique C.
  • Leblanc François
  • Ogino Tatsuki
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118 (6), pp.3233-3242. To examine the effects of planetary surface conductivity and the southward IMF strength on ion dynamics, systematic trajectory tracings of Na⁺ ions were performed in the electric and magnetic field configurations obtained from magnetohydrodynamics (MHD) simulations of the solar wind-Mercury interaction. Comparison with a previous study, which used an analytical model that rescaled the Earth's magnetosphere and assumed the existence of the distant neutral line (DNL) in Mercury's magnetotail, shows a drastic change in the Na⁺ precipitation pattern onto due to the formation of the near-Mercury neutral line (NMNL) in MHD simulations. The Na⁺ precipitation band at approximately 30 degrees of latitude (LAT), which was obtained in the previous study, disappeared in the equivalent low-conductivity MHD case due to the NMNL formation, while the NMNL formation causes high-energy Na⁺ precipitation in the equatorial region. The change in strength of the southward IMF (sBz) alters the location of the NMNL and the Na⁺ precipitation pattern. In the low-conductivity sBz = 5 case, both the equatorial precipitation and the Na⁺ band at approximately LAT = 30 are formed. In the high-conductivity sBz = 5 case, magnetospheric convection through the polar regions is suppressed, which results in a region of dense Na⁺ near the planet. These results suggest that the precipitation pattern of planetary ions onto Mercury's surface changes significantly with the activity level of Mercury's magnetosphere. It is also suggested that observations of the magnetospheric convection, the distribution of Na⁺ ions around the planet, or the precipitation pattern of Na⁺ ions onto the planetary surface can provide us information about the surface conductivity. (10.1002/jgra.50181)
  DOI : 10.1002/jgra.50181
• Study of reconnection physics using laser-generated B fields
  
  • Smets Roch
  • Belmont Gérard
  • Aunai N.
  • Fuchs J. C.
  • Boniface C.
  • Aulanier G.
  , 2013.
• Commutation rapide déclenchée par filamentation laser femtoseconde
  
  • Larour Jean
  • Arantchouk Léonid
  • Houard Aurélien
  Flash X - La revue scientifique de l'Ecole polytechnique, Ecole polytechnique, 2013, 15, pp.55-57. La revue scientifique de l'Ecole polytechnique (parution annuelle) ISSN : 1775-0385 Le phénomène de filamentation laser dans lair a été décrit dans un précédent numéro (Flash X n° 12) par A. Houard et A. Mysyrowicz, chercheurs du LOA (Laboratoire dOptique appliquée). Rappelons ici quil apparaît spontanément le long dun faisceau laser de durée femtoseconde (fs) quand sa puissance dépasse un seuil critique de quelques GW. un équilibre dynamique entre la diffraction naturelle du faisceau, leffet Kerr, et la défocalisation par lair ionisé, maintient lintensité dans le coeur du faisceau sur une distance qui peut dépasser un mètre, entraînant la formation dun canal de plasma dans le sillage de limpulsion. Le point de démarrage, la longueur des canaux de plasma et leur distribution transverse sont contrôlables en jouant sur les paramètres de limpulsion laser initiale (énergie, durée, diamètre du faisceau).
• Simulation benchmarks for low-pressure plasmas: Capacitive discharges
  
  • Turner M.M.
  • Derzsi A.
  • Donkó Z.
  • Eremin D.
  • Kelly S.J.
  • Lafleur Trevor
  • Mussenbrock T.
  Physics of Plasmas, American Institute of Physics, 2013, 20, pp.013507. Benchmarking is generally accepted as an important element in demonstrating the correctness of computer simulations. In the modern sense, a benchmark is a computer simulation result that has evidence of correctness, is accompanied by estimates of relevant errors, and which can thus be used as a basis for judging the accuracy and efficiency of other codes. In this paper, we present four benchmark cases related to capacitively coupled discharges. These benchmarks prescribe all relevant physical and numerical parameters. We have simulated the benchmark conditions using five independently developed particle-in-cell codes. We show that the results of these simulations are statistically indistinguishable, within bounds of uncertainty that we define. We, therefore, claim that the results of these simulations represent strong benchmarks, which can be used as a basis for evaluating the accuracy of other codes. These other codes could include other approaches than particle-in-cell simulations, where benchmarking could examine not just implementation accuracy and efficiency, but also the fidelity of different physical models, such as moment or hybrid models. We discuss an example of this kind in the Appendix. Of course, the methodology that we have developed can also be readily extended to a suite of benchmarks with coverage of a wider range of physical and chemical phenomena. (10.1063/1.4775084)
  DOI : 10.1063/1.4775084
• Anomalous collisionality in low-pressure plasmas
  
  • Lafleur Trevor
  • Chabert Pascal
  • Turner M.M.
  • Booth Jean-Paul
  Physics of Plasmas, American Institute of Physics, 2013, 20 (12), pp.124503. Based on a theoretical argument from fundamental kinetic theory, by way of simple worked examples, and through the use of particle-in-cell simulations of capacitively coupled plasmas, we demonstrate that conventional methods for calculating the momentum transfer collision frequency in low-pressure plasmas can be seriously erroneous. This potentially plays an important and previously unconsidered role in many low-pressure discharges, and at least in part provides a possible explanation for anomalous behaviour often encountered in these plasmas. (10.1063/1.4859155)
  DOI : 10.1063/1.4859155
• Action diffusion and lifetimes of quasistationary states in the Hamiltonian Mean Field model
  
  • Ettoumi Wahb
  • Firpo Marie-Christine
  Physical Review E, American Physical Society (APS), 2013, 87, pp.030102(R). Out-of-equilibrium quasistationary states (QSSs) are one of the signatures of a broken ergodicity in long-range interacting systems. For the widely studied Hamiltonian Mean-Field model, the lifetime of some QSSs has been shown to diverge with the number N of degrees of freedom with a puzzling N¹.7 scaling law, contradicting the otherwise widespread N scaling law. It is shown here that this peculiar scaling arises from the locality properties of the dynamics captured through the computation of the diffusion coefficient in terms of the action variable. The use of a mean first passage time approach proves to be successful in explaining the non-trivial scaling at stake here, and sheds some light on another case, where lifetimes diverging as e^N above some critical energy have been reported. (10.1103/PhysRevE.87.030102)
  DOI : 10.1103/PhysRevE.87.030102
• Theory for the self-bias formation in capacitively coupled plasmas excited by arbitrary waveforms
  
  • Lafleur Trevor
  • Chabert Pascal
  • Turner M.M.
  • Booth Jean-Paul
  Plasma Sources Science and Technology, IOP Publishing, 2013, 22 (6), pp.065013. We develop a semi-analytical theory for the self-bias formation in capacitively coupled plasmas excited by arbitrary radio-frequency (rf) waveforms. The requirement of rf current continuity and voltage balance across the discharge results in the need for a self-bias voltage to develop with non-sinusoidal excitations, even in geometrically symmetric systems. The theory is compared extensively with a wide range of experimental and particle-in-cell (PIC) simulation data within the literature, and is found to be in excellent agreement. Furthermore, it is shown that the present theory is formally equivalent to the original model proposed by Heil et al (2008 J. Phys. D: Appl. Phys. 41 165202), but goes further by explicitly allowing the time-varying sheath voltages and symmetry parameter to be evaluated without input from PIC simulations. (10.1088/0963-0252/22/6/065013)
  DOI : 10.1088/0963-0252/22/6/065013
• Capacitively coupled radio-frequency plasmas excited by tailored voltage waveforms
  
  • Lafleur Trevor
  • Delattre Pierre-Alexandre
  • Johnson E.V.
  • Booth Jean-Paul
  Plasma Physics and Controlled Fusion, IOP Publishing, 2013, 55 (12), pp.124002. By applying certain types of ?tailored? voltage waveforms (TVWs) to capacitively coupled plasmas, a dc self-bias and an asymmetric plasma response can be produced, even in geometrically symmetric reactors. Furthermore, these arbitrary applied waveforms can produce a number of interesting phenomena that are not present in typical single-frequency sinusoidal discharges. This electrical asymmetry effect presents emerging possibilities for the improved control of the ion energy and ion flux in these systems; parameters of vital importance to both etching and deposition applications for materials processing. With a combined research approach utilizing both experimental measurements, and particle-in-cell simulations, we review and extend recent investigations that study a particular class of TVW. The waveforms used have a pulse-type shape and are composed of a varying number of harmonic frequencies. This allows a strong self-bias to be produced, and causes most of the applied voltage to be dropped across a single sheath. Additionally, decreasing the pulse width (by increasing the number of harmonics), allows the plasma density and ion flux to be increased. Simulation and experimental results both demonstrate that this type of waveform can be used to separately control the ion flux and ion energy, while still producing a uniform plasma over large area (50 cm diameter) rf electrodes. (10.1088/0741-3335/55/12/124002)
  DOI : 10.1088/0741-3335/55/12/124002
• Statistical properties of planetary heavy-ion precipitations toward the Martian ionosphere obtained from Mars Express
  
  • Hara T.
  • Seki K.
  • Futaana Y.
  • Yamauchi M.
  • Barabash S.
  • Fedorov A. O.
  • Yagi M.
  • Delcourt Dominique C.
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118 (8), pp.5348-5357. The interplanetary magnetic field (IMF) embedded in the solar wind interacts with the Martian crustal magnetic field and atmosphere. The IMF orientation is one of the important parameters to control the acceleration and precipitation of planetary heavy ions (PHIs). We statistically investigate the effects of the IMF orientation on PHI precipitations toward the ionosphere based on observations by Mars Express (MEX). We identified 59 PHI precipitation events between July 2007 and September 2009. To estimate the IMF orientation without magnetometer that MEX does not carry, we used the velocity distribution of exospheric-origin pickup protons. We estimated the IMF orientation without its polarity for 10 events. The results show that the precipitations of PHIs tend to be observed around pole regions in the MSE (Mars-centered, solar electrical) coordinates determined from the solar wind electric field (Esw), in which the pole axis directs to the parallel or antiparallel to Esw due to the ambiguity in the IMF polarity determination. The observed precipitating PHIs are accelerated only up to a few keV. This feature may reflect the short distance from the picked-up region. For one of these 10 events, we estimated the IMF polarity by comparing the velocity distribution of exospheric-origin pickup protons observed by MEX with those obtained from statistical trajectory tracing simulations under two cases of possible IMF polarity conditions. The estimated polarity indicates that the PHI precipitation in this event is observed in the downward electric field hemisphere in MSE, where Esw points to Mars in the pole region. (10.1002/jgra.50494)
  DOI : 10.1002/jgra.50494
• Structures of dayside whistler-mode waves deduced from conjugate diffuse aurora
  
  • Nishimura Y.
  • Bortnik J.
  • Li W.
  • Thome R.M.
  • Ni B.
  • Lyons L.R.
  • Angelopoulos V.
  • Ebihara Y.
  • Bonnell J. W.
  • Le Contel Olivier
  • Auster U.
  Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2013, 118 (2), pp.664-673. [1] We present simultaneous measurements of dayside diffuse aurora and whistler-mode waves made by the South Pole all-sky imager and two of the THEMIS spacecraft. We found a high correlation between the diffuse aurora intensity at 557.7&#8201;nm near the footprint latitudes of THEMIS and whistler-mode wave intensity measured on board. The power in other wave modes was negligibly small in most cases, indicating that the dayside diffuse aurora is driven by precipitating energetic electrons resonating with whistler-mode waves. The high correlation over a wide L* range (6&#8201;<&#8201;L*&#8201;<&#8201;11) further allowed us to magnetically link the wave and magnetospheric plasma distributions with the auroral patterns. Two distinct regions of whistler-mode waves and ambient plasma density were found outside the plasmasphere near the equator: (1) intense waves in a smooth, low density and (2) moderate waves with enhanced and fluctuating density. The whistler-mode wave intensity in the fluctuating plasma density region is positively correlated with the ambient density variations. The corresponding auroral images show an azimuthally elongated diffuse auroral band on the field lines connected to the low density region, as opposed to a structured diffuse aurora on the fluctuating density field lines. Each structured diffuse auroral patch was stable for a few tens of minutes and slowly drifted azimuthally. The high correlation of waves and auroras indicates that the structured diffuse auroral pattern reflects the spatial distribution of whistler-mode waves and ambient plasma density in space. The enhanced density measured by the spacecraft is quasi-spatial and contributes to enhanced growth of whistler-mode waves. (10.1029/2012JA018242)
  DOI : 10.1029/2012JA018242
• Interaction of plasma transport and turbulence on particle fuelling
  
  • Tamain Patrick
  • Bonhomme Gérard
  • Brochard Frédéric
  • Clairet Frédéric
  • Gil C.
  • Gunn J.
  • Hennequin P.
  • Hornung G.
  • Segui J. L.
  • Vermare L.
  • Ghendrih Philippe
  • Team Tore Supra
  Journal of Nuclear Materials, Elsevier, 2013, 438 (S), pp.S148-S154. We report the results of an experimental investigation of the impact of Supersonic Molecular Beam Injection in the Tore Supra tokamak. Several diagnostics were synchronised with the injection to extract a global picture of the physics at play from the time scale of turbulence (similar to 10 mu s) to the full-recovery time (similar to 1 s). As previously reported, a strong impact of the injection on density and temperature profiles is observed. Both fields exhibit a complex dynamic response involving different phases and time scales. In particular, we show that the effective particle fuelling efficiency is determined by a period of degraded confinement that follows the injection, during which the edge density collapses, in some cases, lower than the initial one. This phase is characterised by a dramatic change in the turbulent transport, with a drop of the frequency spectrum and the observation of large coherent structures as opposed to small intermittent fluctuations before the injection. (10.1016/j.jnucmat.2013.01.023)
  DOI : 10.1016/j.jnucmat.2013.01.023
• A study of helium atmospheric-pressure guided streamers for potential biological applications
  
  • Gazeli Kristacq
  • Noel Cédric
  • Clement Franck
  • Dauge C.
  • Svarnas P.
  • Belmonte Thierry
  Plasma Sources Science and Technology, IOP Publishing, 2013, 22 (2), pp.025020. The origin of differences in the rotational temperatures of various molecules and ions (N-2(+)(B), OH(A) and N-2(C)) is studied in helium atmospheric-pressure guided streamers. The rotational temperature of N-2(+)(B) is room temperature. It is estimated from the emission band of the first negative system at 391.4 nm, and it is governed by the temperature of N-2(X) in the surrounding air. N-2(X) is ionized by direct electron impact in the outer part of the plasma. N-2(+)(B) is deactivated by collisions with N-2 and O-2. The rotational temperature of OH(A), estimated from the OH band at 306.4 nm, is slightly higher than that of N-2(+)(B). OH(A) is excited by electron impact with H2O during the first 100 ns of the applied voltage pulse. Next, OH(A) is produced by electron impact with OH(X) created by the quenching of OH(A) by N-2 and O-2. H2O diffuses deeper than N-2 into the plasma ring and the rotational temperature of OH(A) is slightly higher than that of N-2(+)(B). The rotational temperature of N-2(C), estimated from the emission of the second positive system at 315.9 nm, is governed by its collisions with helium. The gas temperature of helium at the beginning of the pulse is predicted to be several hundred kelvin higher than room temperature. (10.1088/0963-0252/22/2/025020)
  DOI : 10.1088/0963-0252/22/2/025020
• Cell death induced on cell cultures and nude mouse skin by non-thermal, nanosecond-pulsed generated plasma
  
  • Duval Arnaud
  • Marinov Ilya
  • Bousquet Guilhem
  • Gapihan Guillaume
  • Starikovskaia Svetlana
  • Rousseau Antoine
  • Janin Anne
  PLoS ONE, Public Library of Science, 2013, 8 (12), pp.e83001. Non-thermal plasmas are gaseous mixtures of molecules, radicals, and excited species with a small proportion of ions and energetic electrons. Non-thermal plasmas can be generated with any high electro-magnetic field. We studied here the pathological effects, and in particular cell death, induced by nanosecond-pulsed high voltage generated plasmas homogeneously applied on cell cultures and nude mouse skin. In vitro, Jurkat cells and HMEC exhibited apoptosis and necrosis, in dose-dependent manner. In vivo, on nude mouse skin, cell death occurred for doses above 113 J/cm(2) for the epidermis, 281 J/cm(2) for the dermis, and 394 J/cm(2) for the hypodermis. Using electron microscopy, we characterized apoptosis for low doses and necrosis for high doses. We demonstrated that these effects were not related to thermal, photonic or pH variations, and were due to the production of free radicals. The ability of cold plasmas to generate apoptosis on cells in suspension and, without any sensitizer, on precise skin areas, opens new fields of application in dermatology for extracorporeal blood cell treatment and the eradication of superficial skin lesions. (10.1371/journal.pone.0083001)
  DOI : 10.1371/journal.pone.0083001
• Hysteresis effects in the formation of a neutralizing beam plasma at low ion energy
  
  • Rafalskyi D.V.
  • Aanesland Ane
  EPL - Europhysics Letters, European Physical Society / EDP Sciences / Società Italiana di Fisica / IOP Publishing, 2013, 104 (3), pp.35004. In this paper, the PEGASES II thruster prototype is used as an ion source generating low-energy positive Ar ion beam, extracted without an external neutralizer. The ions are extracted and accelerated from the source using a two-grid system. The extracted positive ion beam current is measured on a large beam target that can be translated along the acceleration axis. The ion beam current shows a stepwise transition from a low-current to a high-current extraction regime with hysteresis. The hysteresis region depends strongly upon the beam target position. Langmuir probe measurements in the plume show high plasma potentials and low plasma densities in the low-current mode, while the plasma potential drops and the density increases in the high-current mode. The ion energy distribution functions of the beam are measured for different regimes of ion extraction. The ion beam extracted in the high-current mode is indicated by the presence of an additional low-energy peak corresponding to ions from an ion-beam plasma created in the downstream chamber, as well as 1020 times higher intensity of the primary ion beam peak. The hysteresis behavior is explained by the formation of a downstream neutralizing beam plasma, that depends on the target position and pressure in agreement with a Paschen-like breakdown by secondary electrons. The obtained results are of high relevance for further development of the PEGASES thruster, as well as for improving existing neutralizer-free concepts of the broad-beam ion sources. (10.1209/0295-5075/104/35004)
  DOI : 10.1209/0295-5075/104/35004
• Controlled deposition of sulphur-containing semiconductor and dielectric nano-structured films on metals in SF<SUB>6</SUB> ion-ion plasma
  
  • Rafalskyi D.V.
  • Bredin Jérôme
  • Aanesland Ane
  Journal of Applied Physics, American Institute of Physics, 2013, 114 (21), pp.213303. In the present paper, the deposition processes and formation of films in SF6 ion-ion plasma, with positive and negative ion flows accelerated to the surface, are investigated. The PEGASES (acronym for Plasma Propulsion with Electronegative GASES) source is used as an ion-ion plasma source capable of generating almost ideal ion-ion plasma with negative ion to electron density ratio more than 2500. It is shown that film deposition in SF6 ion-ion plasma is very sensitive to the polarity of the incoming ions. The effect is observed for Cu, W, and Pt materials. The films formed on Cu electrodes during negative and positive ion assisted deposition were analyzed. Scanning electron microscope analysis has shown that both positive and negative ion fluxes influence the copper surface and leads to film formation, but with different structures of the surface: the low-energy positive ion bombardment causes the formation of a nano-pored film transparent for ions, while the negative ion bombardment leads to a continuous smooth insulating film. The transversal size of the pores in the porous film varies in the range 50500&#8201;nm, and further analysis of the film has shown that the film forms a diode together with the substrate preventing positive charge drain, and positive ions are neutralized by passing through the nano-pores. The film obtained with the negative ion bombardment has an insulating surface, but probably with a multi-layer structure: destroying the top surface layer allows to measure similar diode IV-characteristics as for the nano-pored film case. Basing on results, practical conclusions for the probes and electrodes cleaning in ion-ion SF6 plasmas have been made. Different applications are proposed for the discovered features of the controlled deposition from ion-ion plasmas, from Li-sulphur rechargeable batteries manufacturing and nanofluidics issues to the applications for microelectronics, including low-k materials formation. (10.1063/1.4842915)
  DOI : 10.1063/1.4842915
• On the reactivity of plasma-treated photo-catalytic TiO<SUB>2</SUB> surfaces for oxidation of C<SUB>2</SUB>H<SUB>2</SUB> and CO
  
  • Lopatik D.
  • Marinov Daniil
  • Guaitella Olivier
  • Rousseau Antoine
  • Roepcke J.
  Journal of Physics D: Applied Physics, IOP Publishing, 2013, 46, pp.255203. The objective of this study is to understand fundamental aspects of interactions of plasmas with catalytic surfaces. Based on this approach the reactivity of plasma treated and stimulated catalytic surfaces of TiO2 is studied by analysing the oxidation (i) of C2H2 to CO and CO2 and (ii) of CO to CO2. The inner surface of a Pyrex discharge tube is coated with TiO2 films impregnated with TiO2 nanoparticles, which provides a surface area of about 4 m2. In addition to the exposure of the TiO2 surface by low-pressure radio-frequency plasmas using O2, Ar or N2 (f = 13.56 MHz, p = 0.53 mbar, P = 17 W) the surfaces are stimulated by heating and UV radiation treatment. The temporal development of the concentrations of the precursor gases C2H2 or CO and of the reaction products is monitored using quantum cascade laser absorption spectroscopy, which provides multi-component detection in the mid-infrared spectral range. The C2H2 concentration was found to be nearly constant over time after a pre-treatment with Ar or N2 discharges using an initial gas mixture of 1% C2H2 in Ar. However, a strong decay of the concentration of C2H2 is observed for pure O2 plasma pre-treatment. In general, the decay is found to be nearly exponential with time constant in the order of about 10 min. The reactive adsorption of C2H2 molecules on the inner surface of the tube reactor showed a density of about 7.5 × 1012 C2H2 molecules cm&#8722;2. This behaviour demonstrates that the reaction (\rm O_\rm ads \rm C_2 \rm H_2)_\rm TiO_2 produces some adsorbed intermediates, which can be thermally or photo-catalytically oxidized to CO2. In contrast, when 1% CO in Ar is used as an initial gas mixture no adsorption processes on the TiO2 surface could be detected. An effective destruction of CO took part via photo-catalytic oxidation. (10.1088/0022-3727/46/25/255203)
  DOI : 10.1088/0022-3727/46/25/255203
• Fine-structure-resolved electron collisions from chlorine atoms in the (3p<SUP>5</SUP>)<SUP>2</SUP>P<SUB>3/2</SUB><SUP>o</SUP> and (3p<SUP>5</SUP>)<SUP>2</SUP>P<SUB>1/2</SUB><SUP>o</SUP> states
  
  • Wang Yang
  • Zatsarinny Oleg
  • Bartschat Klaus
  • Booth Jean-Paul
  Physical Review A : Atomic, molecular, and optical physics [1990-2015], American Physical Society, 2013, 87, pp.022703. The B-spline R-matrix method is employed to calculate elastic electron scattering from chlorine atoms in the (3p5)2P3/2,1/2o states and electron-induced collisions between these two finestructure levels. The polarizability of the target states is accounted for by including polarized pseudostates in the close-coupling expansion, while relativistic effects are treated at the level of the semirelativistic Breit-Pauli approximation. We find the Ramsauer minimum in the elastic channels at a significantly lower projectile energy (&#8776;0.2 eV) than previous calculations, due to an apparent strong sensitivity of the theoretical predictions on the details of the model, especially the target structure. The present results are relevant to the determination of chlorine atomic densities in Cl2-containing industrial plasma etch reactors. (10.1103/PhysRevA.87.022703)
  DOI : 10.1103/PhysRevA.87.022703
• Transport of radial heat flux and second sound in fusion plasmas
  
  • Gürcan Özgür D.
  • Diamond P.H.
  • Garbet X.
  • Berionni Vincent
  • Dif-Pradalier Guilhem
  • Hennequin Pascale
  • Morel Pierre
  • Kosuga Y.
  • Vermare Laure
  Physics of Plasmas, American Institute of Physics, 2013, 20, pp.022307. Simple flux-gradient relations that involve time delay and radial coupling are discussed. Such a formulation leads to a rather simple description of avalanches and may explain breaking of gyroBohm transport scaling. The generalization of the flux-gradient relation (i.e., constitutive relation), which involve both time delay and spatial coupling, is derived from drift-kinetic equation, leading to kinetic definitions of constitutive elements such as the flux of radial heat flux. This allows numerical simulations to compute these cubic quantities directly. The formulation introduced here can be viewed as an extension of turbulence spreading to include the effect of spreading of cross-phase as well as turbulence intensity, combined in such a way to give the flux. The link between turbulence spreading and entropy production is highlighted. An extension of this formulation to general quasi-linear theory for the distribution function in the phase space of radial position and parallel velocity is also discussed. (10.1063/1.4792161)
  DOI : 10.1063/1.4792161